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Benedetti, A, Reid, JS, Baklanov, A et al. (26 more authors) (2018) Status and future of Numerical Atmospheric Aerosol Prediction with a focus on data requirements. Atmospheric Chemistry and Physics Discussions. ISSN 1680-7367
Abstract
Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centres due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation and military authorities, solar energy plant
managers, providers of climate services, and health professionals. The prediction of aerosol particle 5 properties in Numerical Weather prediction (NWP) models faces a number of challenges owing to
the complexity of atmospheric aerosol processes and their sensitivity to the underlying meteorological conditions. Errors in aerosol prediction concern all processes involved in the aerosol life cycle. These include errors on the source terms (for both anthropogenic and natural emissions), errors directly dependent on the meteorology (e.g., mixing, transport, scavenging by precipitation), as well 10 as errors related to aerosol chemistry (e.g., nucleation, gas-aerosol partitioning, chemical transformation and growth, hygroscopicity). The main goal of current research on aerosol forecast consists in prioritizing these errors and trying to reduce the most important ones through model development
and data assimilation. Aerosol particle observations from satellite and ground-based platforms have been crucial to guide model development of the recent years, and have been made more readily 15 available for model evaluation and assimilation. However, for the sustainability of the aerosol particle prediction activities around the globe, it is crucial that quality aerosol observations continue to be made available from different platforms (space, near-surface, and aircraft) and freely shared. This
white paper reviews current requirements for aerosol observations in the context of the operational activities carried out at various global and regional centres. Some of the requirements are equally applicable to aerosol-climate research. However, the focus here is on the global operational prediction of aerosol properties such as mass concentrations and optical parameters. Most operational models are based on bulk schemes that do not predict the size distribution of the aerosol particles. Others are based on a mix of “bin” and bulk schemes with limited capability to simulate the size information. However the next generation of aerosol operational models will have the capability to predict both
25 mass and number density which will provide a more complete description of the aerosols properties. A brief overview of the state-of-the-art is provided with an introduction on the importance of aerosol
prediction activities. The criteria on which the requirements for aerosol observations are based are also outlined. Assimilation and evaluation aspects are discussed from the perspective of the user requirements.
Metadata
Item Type: | Article |
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Authors/Creators: |
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Copyright, Publisher and Additional Information: | © Author(s) 2018. This is an open access discussion paper under the terms of the Creative Commons Attribution License (CC-BY 4.0). |
Dates: |
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Institution: | The University of Leeds |
Academic Units: | The University of Leeds > Faculty of Environment (Leeds) > School of Earth and Environment (Leeds) > Inst for Climate & Atmos Science (ICAS) (Leeds) |
Funding Information: | Funder Grant number NERC NE/L005352/1 |
Depositing User: | Symplectic Publications |
Date Deposited: | 20 Sep 2018 09:03 |
Last Modified: | 23 May 2022 13:55 |
Status: | Published |
Publisher: | European Geosciences Union |
Identification Number: | 10.5194/acp-2018-42 |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:131725 |
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Status and future of Numerical Atmospheric Aerosol Prediction with a focus on data requirements. (deposited 20 Sep 2018 09:03)
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- Status and future of Numerical Atmospheric Aerosol Prediction with a focus on data requirements. (deposited 05 Jul 2018 16:19)