Zhang, Y, Ma, CY, Liu, JJ et al. (2 more authors) (2014) Modelling and simulation of counter-current reactors for continuous hydrothermal flow synthesis of nanoparticles. Dalian Ligong Daxue Xuebao/Journal of Dalian University of Technology, 54 (6). pp. 662-675. ISSN 1000-8608
Abstract
Numerical simulation using computational fluid dynamics is carried out to study the performance of a counter-current reactor in a continuous hydrothermal system for nanomaterial synthesis that is operated under supercritical water condition.Inlet flowrate and temperature are the key process variables and vary in the simulation.The predicted temperatures are in good agreement with measurements taken from a laboratory rig of identical design and under the same operating conditions.It is found that fast mixing in the reactor can be achieved by high inlet temperature,high inlet flowrate of the supercritical water and using unbalanced flow conditions,i.e.the supercritical water flowrate should not be equal to that of the precursor.The comparative simulation also reveals that the insertion length of the inner tube is a key factor dictating the reactor performance,and it needs to be less than 72.5 mm in order to achieve satisfactory mixing under the current reactor configuration.
Metadata
Item Type: | Article |
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Authors/Creators: |
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Keywords: | counter-current reactor; hydrothermal synthesis of nanomaterials; computational fluid dynamics; supercritical water; mixing; reactor design |
Dates: |
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Institution: | The University of Leeds |
Academic Units: | The University of Leeds > Faculty of Engineering & Physical Sciences (Leeds) > School of Chemical & Process Engineering (Leeds) > Institute for Particle Science and Engineering (Leeds) The University of Leeds > Faculty of Environment (Leeds) > School of Earth and Environment (Leeds) > Inst of Geophysics and Tectonics (IGT) (Leeds) |
Depositing User: | Symplectic Publications |
Date Deposited: | 31 Mar 2016 08:20 |
Last Modified: | 31 Mar 2016 08:53 |
Status: | Published |
Publisher: | Dalian University of Technology |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:93094 |