Califano, M. (2007) Giant suppression of Auger electron cooling in charged nanocrystals. Applied Physics Letters, 91 (17). p. 172114. ISSN 00036951
Abstract
This letter presents a detailed study of the electron relaxation lifetimes from the excited p-like state into the ground s-like state via Auger cooling in positively and negatively charged CdSe nanocrystals, where the dependence of Auger cooling rates on size, temperature and carrier-carrier interaction effects is investigated. A nearly two-orders-of-magnitude reduction of Auger rates is found in small nanocrystals populated by two electrons and one hole at room temperature. This effect increases with decreasing temperature leading to a total lifetime increase of up to 4 orders of magnitude for T ∼ 10 K. Such a giant suppression of Auger cooling rates appears to be a general property of semiconductor nanocrystals. A similar reduction of Auger rates at room T is found in negatively charged PbSe nanocrystals as well.
Metadata
Item Type: | Article |
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Authors/Creators: |
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Copyright, Publisher and Additional Information: | © 2007 American Institute Physics. This is an author produced version of a paper published in Applied Physics Letters. Uploaded in accordance with the publisher's self-archiving policy. |
Dates: |
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Institution: | The University of Leeds |
Academic Units: | The University of Leeds > Faculty of Engineering & Physical Sciences (Leeds) > School of Electronic & Electrical Engineering (Leeds) > Pollard Institute (Leeds) |
Depositing User: | Sherpa Assistant |
Date Deposited: | 18 Dec 2007 16:47 |
Last Modified: | 16 Sep 2016 13:33 |
Published Version: | http://dx.doi.org/10.1063/1.2803296 |
Status: | Published |
Publisher: | American Institute of Physics |
Identification Number: | 10.1063/1.2803296 |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:3543 |