Long, Y., Chen, Z., Wu, L. et al. (6 more authors) (2024) Electrocatalytic CO2 reduction to alcohols: progress and perspectives. Small Science, 4 (8). 2400129. ISSN 2688-4046
Abstract
Utilizing renewable electricity for the electrocatalytic conversion of CO2 into alcohols represents a promising avenue for generating value-added fuels and achieving carbon neutrality. Recently, there has been growing scientific interest in achieving high-efficiency conversion of CO2 to alcohols, with significant advancements made in mechanism understanding, reactor design, catalyst development, and more. Herein, a thorough examination of the latest advances in electrocatalytic CO2 reduction reaction (CO2RR) to alcohols is provided. General mechanisms and pathways of electrocatalytic conversion of CO2-to-alcohols are systematically illustrated. Subsequently, electrolyzer configurations, electrolytes, and electrocatalysts employed in CO2RR are summarized. After that, critical operating parameters (e.g., reaction pressure, temperature, and pH) that would significantly influence the CO2RR process are also analyzed. Finally, the review addresses challenges and offers perspectives in this field to guide future studies aimed at advancing CO2-to-alcohols conversion technologies.
Metadata
Item Type: | Article |
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Authors/Creators: |
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Copyright, Publisher and Additional Information: | © 2024 The Author(s). Small Science published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited (http://creativecommons.org/licenses/by/4.0/). |
Keywords: | Engineering; Materials Engineering; Affordable and Clean Energy; Climate Action |
Dates: |
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Institution: | The University of Sheffield |
Academic Units: | The University of Sheffield > Faculty of Engineering (Sheffield) > Department of Chemical and Biological Engineering (Sheffield) |
Depositing User: | Symplectic Sheffield |
Date Deposited: | 04 Jul 2024 15:05 |
Last Modified: | 04 Oct 2024 16:13 |
Status: | Published |
Publisher: | Wiley |
Refereed: | Yes |
Identification Number: | 10.1002/smsc.202400129 |
Related URLs: | |
Sustainable Development Goals: | |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:214192 |