Pardikar, K. orcid.org/0000-0001-5720-6518, Entwistle, J., Ge, R. et al. (2 more authors) (2023) Status and outlook for lithium-ion battery cathode material synthesis and the application of mechanistic modeling. Journal of Physics: Energy, 5 (2). 022002. ISSN 2515-7655
Abstract
This work reviews different techniques available for the synthesis and modification of cathode active material (CAM) particles used in Li-ion batteries. The synthesis techniques are analyzed in terms of processes involved and product particle structure. The knowledge gap in the process-particle structure relationship is identified. Many of these processes are employed in other similar industries; hence, parallel insights and knowledge transfer can be applied to battery materials. Here, we discuss examples of applications of different mechanistic models outside the battery literature and identify similar potential applications for the synthesis of CAMs. We propose that the widespread implementation of such mechanistic models will increase the understanding of the process-particle structure relationship. Such understanding will provide better control over the CAM synthesis technique and open doors to the precise tailoring of product particle morphologies favorable for enhanced electrochemical performance.
Metadata
Item Type: | Article |
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Authors/Creators: |
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Copyright, Publisher and Additional Information: | © 2023 The Author(s). This is an Open Access article distributed under the terms of the Creative Commons Attribution Licence (https://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. |
Keywords: | lithium-ion battery; cathode active material synthesis; mechanistic modeling; process-product relationship; process control |
Dates: |
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Institution: | The University of Sheffield |
Academic Units: | The University of Sheffield > Faculty of Engineering (Sheffield) > Department of Chemical and Biological Engineering (Sheffield) |
Funding Information: | Funder Grant number THE FARADAY INSTITUTION EP/T012412/1 |
Depositing User: | Symplectic Sheffield |
Date Deposited: | 22 Jan 2024 16:12 |
Last Modified: | 22 Jan 2024 16:12 |
Status: | Published |
Publisher: | IOP Publishing |
Refereed: | Yes |
Identification Number: | 10.1088/2515-7655/acc139 |
Related URLs: | |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:207556 |