This is the latest version of this eprint.
McCoy, DT orcid.org/0000-0003-1148-6475, Bender, FA-M, Grosvenor, DP et al. (4 more authors) (2018) Predicting decadal trends in cloud droplet number concentration using reanalysis and satellite data. Atmospheric Chemistry and Physics, 18 (3). pp. 2035-2047. ISSN 1680-7316
Abstract
Cloud droplet number concentration (CDNC) is the key state variable that moderates the relationship between aerosol and the radiative forcing arising from aerosol–cloud interactions. Uncertainty related to the effect of anthropogenic aerosol on cloud properties represents the largest uncertainty in total anthropogenic radiative forcing. Here we show that regionally averaged time series of the Moderate-Resolution Imaging Spectroradiometer (MODIS) observed CDNC of low, liquid-topped clouds is well predicted by the MERRA2 reanalysis near-surface sulfate mass concentration over decadal timescales. A multiple linear regression between MERRA2 reanalyses masses of sulfate (SO₄), black carbon (BC), organic carbon (OC), sea salt (SS), and dust (DU) shows that CDNC across many different regimes can be reproduced by a simple power-law fit to near-surface SO₄, with smaller contributions from BC, OC, SS, and DU. This confirms previous work using a less sophisticated retrieval of CDNC on monthly timescales. The analysis is supported by an examination of remotely sensed sulfur dioxide (SO₂) over maritime volcanoes and the east coasts of North America and Asia, revealing that maritime CDNC responds to changes in SO₂ as observed by the ozone monitoring instrument (OMI). This investigation of aerosol reanalysis and top-down remote-sensing observations reveals that emission controls in Asia and North America have decreased CDNC in their maritime outflow on a decadal timescale.
Metadata
Item Type: | Article |
---|---|
Authors/Creators: |
|
Copyright, Publisher and Additional Information: | © Author(s) 2018. This work is distributed under the Creative Commons Attribution 4.0 License. |
Dates: |
|
Institution: | The University of Leeds |
Academic Units: | The University of Leeds > Faculty of Environment (Leeds) > School of Earth and Environment (Leeds) > Inst for Climate & Atmos Science (ICAS) (Leeds) |
Funding Information: | Funder Grant number EU - European Union GA 641727 |
Depositing User: | Symplectic Publications |
Date Deposited: | 07 Mar 2018 08:54 |
Last Modified: | 01 Nov 2018 11:03 |
Status: | Published |
Publisher: | European Geosciences Union |
Identification Number: | 10.5194/acp-18-2035-2018 |
Open Archives Initiative ID (OAI ID): | oai:eprints.whiterose.ac.uk:128216 |
Available Versions of this Item
-
Predicting decadal trends in cloud droplet number concentration using reanalysis and satellite data. (deposited 01 Nov 2018 11:04)
- Predicting decadal trends in cloud droplet number concentration using reanalysis and satellite data. (deposited 07 Mar 2018 08:54) [Currently Displayed]