High Purcell factor generation of coherent on-chip single photons

On-chip single-photon sources are key components for integrated photonic quantum technologies. Semiconductor quantum dots can exhibit near-ideal single photon emission but suffer from significant dephasing in on-chip geometries owing to nearby etched surfaces. A long-proposed solution is to use the Purcell effect of an optical nanocavity to reduce the radiative lifetime to much less than dephasing timescales. However, until now only modest Purcell enhancements have been observed. Here we use resonant excitation to eliminate slow relaxation paths, revealing a highly Purcell-enhanced radiative lifetime of only 22.7 ps. This is measured by applying a novel high-time-resolution double $\pi$-pulse resonance fluorescence technique to a quantum dot in a waveguide-coupled photonic crystal cavity. Coherent scattering measurements confirm the short lifetime and show that the quantum dot exhibits near-radiatively-limited coherence. Under $\pi$-pulse excitation, the waveguide coupling enables demonstration of an on-chip, on-demand single-photon source exhibiting high purity and indistinguishability without spectral filtering.