Dynamical mechanisms for the recent ozone depletion in the Arctic stratosphere linked to North Pacific sea surface temperatures

The stratospheric ozone layer, which prevents solar ultraviolet radiation from reaching the surface and thereby protects life on earth, is expected to recover from past depletion during this century due to the impact of the Montreal Protocol. However, how the ozone column over the Arctic will evolve over the next few decades is still under debate. In this study, we found that the ozone level in the Arctic stratosphere at 100–150 hPa during 1998–2018 exhibits a decreasing trend of − 0.12 ± 0.07 ppmv decade–1 from MERRA2, suggesting a continued depletion during this century. About 30% of this ozone depletion is contributed by the second leading mode of sea surface temperature anomalies (SSTAs) over the North Pacific with one month leading and therefore is dynamical in origin. The North Pacific SSTAs associated with this mode tend to result in a weakened Aleutian low, a strengthened Western Pacific pattern and a weakened Pacific–North American pattern, which impede the upward propagation of wavenumber-1 waves into the lower stratosphere. The changes in the stratospheric wave activity may result in decreased ozone in the Arctic lower stratosphere through weakening the Brewer-Dobson circulation. Our findings uniquely linked the recent ozone depletion in the Arctic stratosphere to the North Pacific SSTs and might provide new understanding of how dynamical processes control Arctic stratospheric ozone.