Heisenberg pseudo-exchange and emergent anisotropies in field-driven pinwheel artificial spin ice

Rotating all islands in square artificial spin ice (ASI) uniformly about their centers gives rise to the recently reported pinwheel ASI. At angles around 45∘, the antiferromagnetic ordering changes to ferromagnetic and the magnetic configurations of the system exhibit near degeneracy, making it particularly sensitive to small perturbations. We investigate through micromagnetic modeling the influence of dipolar fields produced by physically extended islands in field-driven magnetization processes in pinwheel arrays and compare the results to hysteresis experiments performed in situ using Lorentz transmission electron microscopy. We find that magnetization end states induce a Heisenberg pseudoexchange interaction that governs both the interisland coupling and the resultant array reversal process. Symmetry reduction gives rise to anisotropies and array-corner mediated avalanche reversals through a cascade of nearest-neighbor (NN) islands. The symmetries of the anisotropy axes are related to those of the geometrical array but are misaligned to the array axes as a result of the correlated interactions between neighboring islands. The NN dipolar coupling is reduced by decreasing the island size and, using this property, we track the transition from the strongly coupled regime towards the pure point dipole one and observe modification of the ferromagnetic array reversal process. Our results shed light on important aspects of the interactions in pinwheel ASI and demonstrate a mechanism by which their properties may be tuned for use in a range of fundamental research and spintronic applications.